7–9 Apr 2021
Europe/Stockholm timezone

Investigation of ultrafast charge transfer in push-pull chromophores using table-top soft x-ray HHG spectroscopy

8 Apr 2021, 13:00
1h
ESR Poster ESR Poster Session ESR Poster Session

Speaker

zhuangyan zhang

Description

Pull-push chromophores have the donor acceptor structure where it promotes electrons transfer from electron-rich donor group to electron-deficient acceptor group. It can be linked together by chains of different structures and length such as π-conjugated polyene, which are prototypical systems for intramolecular electron transfer processes. Understanding the dynamics of ultrafast charge transfer processes in donor-acceptor molecular systems generally requires a femtosecond temporal resolution to identify the vibrational coupling modes responsible for the electron transfer and to directly visualize the electronic motions. This project aims to develop and improve the ultra-thin liquid flat-jet and a table-top source of soft X-ray pulses providing photons in the water window (280-540 eV) spectral range, and to perform transient soft X-ray absorption experiments to unravel charge transfer processes in simple acceptor-donor molecular systems in solution.

Primary authors

zhuangyan zhang Erik T. J. Nibbering (Max Born Institute) Arnaud Rouzée (Max Born Institute) Carlo Kleine (Max Born Institute) Marc-Oliver Winghart (Marc-Oliver) Dr Peng Han (Max-Born-Institute)

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