12–14 Aug 2024
Albano Building 3
Europe/Stockholm timezone

Microcavity mediated excitation dynamics of photosynthetic light harvesting complexes

12 Aug 2024, 16:30
30m
Albano Building 3

Albano Building 3

Hannes Alfvéns väg 12, 10691 Stockholm, Sweden
Invited Talk Monday Afternoon

Speaker

Tönu Pullerits (Chemical Physics, Lund University)

Description

Strong light-matter interaction leads to the formation of hybrid polariton states and alters the photophysical dynamics of organic materials and biological systems without modifying their chemical structure. Here, we experimentally investigated a well-known photosynthetic protein, light harvesting 2 complexes (LH2) from purple bacteria under both strong and weak coupling with the light mode of a Fabry-Perot optical microcavity. Using femtosecond pump-probe spectroscopy, we analysed the polariton dynamics of the strongly coupled system. We observed a significant prolongation of the excited state lifetime compared with the bare exciton, which can be explained in terms of the exciton reservoir model. We also demonstrated cavity-mediated excitation transfer between different complexes even in case of weak effective light-mater interaction.

Primary author

Tönu Pullerits (Chemical Physics, Lund University)

Co-authors

Mr Ilmari Rosenkampff (Chemical Physics, Lund University) Dr Daniel Finkelstein Shapiro (Chemical Physics, Lund University) Dr Fan Wu (Chemical Physics, Lund University)

Presentation materials

There are no materials yet.